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Opposite Polarity Surface Photovoltage of MoS2 Monolayers on Au Nanodot versus Nanohole Arrays
- Title
- Opposite Polarity Surface Photovoltage of MoS2 Monolayers on Au Nanodot versus Nanohole Arrays
- Authors
- Song, Jungeun; Kwon, Soyeong; Kim, Bora; Kim, Eunah; Murthy, Lakshmi N. S.; Lee, Taejin; Hong, Inhae; Lee, Byoung Hoon; Lee, Sang Wook; Choi, Soo Ho; Kim, Ki Kang; Cho, Chang-Hee; Hsu, Julia W. P.; Kim, Dong-Wook
- Ewha Authors
- 김동욱; 이상욱; 이병훈
- SCOPUS Author ID
- 김동욱; 이상욱; 이병훈
- Issue Date
- 2020
- Journal Title
- ACS APPLIED MATERIALS & INTERFACES
- ISSN
- 1944-8244
1944-8252
- Citation
- ACS APPLIED MATERIALS & INTERFACES vol. 12, no. 43, pp. 48991 - 48997
- Keywords
- MoS2; localized surface plasmon; surface plasmon polariton; photoluminescence; surface photovoltage
- Publisher
- AMER CHEMICAL SOC
- Indexed
- SCIE; SCOPUS
- Document Type
- Article
- Abstract
- We prepared MoS2 monolayers on Au nanodot (ND) and nanohole (NH) arrays. Both these sample arrays exhibited enhanced photo-luminescence intensity compared with that of a bare SiO2/Si substrate. The reflectance spectra of MoS2/ND and MoS2/NH had clear features originating from excitation of localized surface plasmon and propagating surface plasmon polaritons. Notably, the surface photovoltages (SPV) of these hybrid plasmonic nanostructures had opposite polarities, indicating negative and positive charging at MoS2/ND and MoS2/NH, respectively. Surface potential maps, obtained by Kelvin probe force microscopy, suggested that the potential gradient led to a distinct spatial distribution of photo-generated charges in these two samples under illumination. Furthermore, the local density of photo-generated excitons, as predicted from optical simulations, explained the SPV spectra of MoS2/ND and MoS2/NH. We show that the geometric configuration of the plasmonic nanostructures modified the polarity of photo-generated excess charges in MoS2. These findings point to a useful means of optimizing optoelectronic characteristics and improving the performance of MoS2-based plasmonic devices.
- DOI
- 10.1021/acsami.0c14563
- Appears in Collections:
- 자연과학대학 > 물리학전공 > Journal papers
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