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Facile formation of a meso-meso linked porphyrin dimer catalyzed by a manganese(iv)-oxo porphyrin

Title
Facile formation of a meso-meso linked porphyrin dimer catalyzed by a manganese(iv)-oxo porphyrin
Authors
Takai A.Habermeyer B.Fukuzumi S.
Ewha Authors
Shunichi Fukuzumi
SCOPUS Author ID
Shunichi Fukuzumiscopus
Issue Date
2011
Journal Title
Chemical Communications
ISSN
1359-7345JCR Link
Citation
vol. 47, no. 24, pp. 6804 - 6806
Indexed
SCI; SCIE; SCOPUS WOS scopus
Abstract
A manganese(iv)-oxo porphyrin catalyzes C-C bond formation between zinc porphyrins at the meso-position with a two-electron oxidant to afford the meso-meso linked porphyrin dimer efficiently. The meso-meso linked dimer is formed via formation of the porphyrin radical cation, and the rate-determining step in the catalytic cycle is the formation of a manganese(iv)-oxo porphyrin with a two-electron oxidant. © 2011 The Royal Society of Chemistry.
DOI
10.1039/c1cc10608b
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자연과학대학 > 화학·나노과학전공 > Journal papers
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