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Plasmonic Periodic Nanodot Arrays via Laser Interference Lithography for Organic Photovoltaic Cells with >10% Efficiency

Title
Plasmonic Periodic Nanodot Arrays via Laser Interference Lithography for Organic Photovoltaic Cells with >10% Efficiency
Authors
Oh Y.Lim J.W.Kim J.G.Wang H.Kang B.-H.Park Y.W.Kim H.Jang Y.J.Kim J.Kim D.H.Ju B.-K.
Ewha Authors
김동하Huan Wang
SCOPUS Author ID
김동하scopus; Huan Wangscopus
Issue Date
2016
Journal Title
ACS Nano
ISSN
1936-0851JCR Link
Citation
ACS Nano vol. 10, no. 11, pp. 10143 - 10151
Keywords
laser interference lithographymetal nanodot arrayorganic photovoltaicssurface plasmon
Publisher
American Chemical Society
Indexed
SCIE; SCOPUS WOS scopus
Document Type
Article
Abstract
In this study, we demonstrate a viable and promising optical engineering technique enabling the development of high-performance plasmonic organic photovoltaic devices. Laser interference lithography was explored to fabricate metal nanodot (MND) arrays with elaborately controlled dot size as well as periodicity, allowing spectral overlap between the absorption range of the active layers and the surface plasmon band of MND arrays. MND arrays with ∼91 nm dot size and ∼202 nm periodicity embedded in a poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) hole transport layer remarkably enhanced the average power conversion efficiency (PCE) from 7.52% up to 10.11%, representing one of the highest PCE and degree of enhancement (∼34.4%) levels compared to the pristine device among plasmonic organic photovoltaics reported to date. The plasmonic enhancement mechanism was investigated by both optical and electrical analyses using finite difference time domain simulation and conductive atomic force microscopy studies. © 2016 American Chemical Society.
DOI
10.1021/acsnano.6b05313
Appears in Collections:
자연과학대학 > 화학·나노과학전공 > Journal papers
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