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자연과학대학
화학·나노과학전공
Journal papers
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Direct oxygenation of benzene to phenol using quinolinium ions as homogeneous photocatalysts
Title
Direct oxygenation of benzene to phenol using quinolinium ions as homogeneous photocatalysts
Authors
Ohkubo K.
;
Kobayashi T.
;
Fukuzumi S.
Ewha Authors
Shunichi Fukuzumi
SCOPUS Author ID
Shunichi Fukuzumi
Issue Date
2011
Journal Title
Angewandte Chemie - International Edition
ISSN
1433-7851
Citation
Angewandte Chemie - International Edition vol. 50, no. 37, pp. 8652 - 8655
Indexed
SCI; SCIE; SCOPUS
Document Type
Article
Abstract
Photocatalytic oxygenation of benzene with oxygen and water to phenol has been achieved under ambient conditions by using the 3-cyano-1-methylquinolinium ion as a photocatalyst (see picture). The mechanism was clarified by detecting the π-dimer benzene radical cation produced by photoinduced electron transfer from benzene to the photocatalyst, and by monitoring the reaction of the radical cations with water molecules. Copyright © 2011 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
DOI
10.1002/anie.201102931
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