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자연과학대학
화학·나노과학전공
Journal papers
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Fundamental electron-transfer properties of non-heme oxoiron(IV) complexes
Title
Fundamental electron-transfer properties of non-heme oxoiron(IV) complexes
Authors
Lee Y.-M.
;
Kotani H.
;
Suenobu T.
;
Nam W.
;
Fukuzumi S.
Ewha Authors
남원우
;
이용민
;
Shunichi Fukuzumi
SCOPUS Author ID
남원우
; Shunichi Fukuzumi
; 이용민
Issue Date
2008
Journal Title
Journal of the American Chemical Society
ISSN
0002-7863
Citation
Journal of the American Chemical Society vol. 130, no. 2, pp. 434 - 435
Indexed
SCI; SCIE; SCOPUS
Document Type
Article
Abstract
Electron-transfer kinetics for the reduction of non-heme oxoiron(IV) complexes by a series of ferrocene derivatives were examined in deaerated acetonitrile, and the resulting data were evaluated in light of the Marcus theory of electron transfer to determine the reorganization energies of electron transfer and the one-electron reduction potentials of non-heme oxoiron(IV) complexes. The electron-transfer properties of non-heme oxoiron(IV) complexes are featured by the larger reorganization energies of electron transfer and the lower one-electron reduction potentials as compared with those of heme oxoiron(IV) complexes. Copyright © 2008 American Chemical Society.
DOI
10.1021/ja077994e
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